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  • Received: Mar. 19, 2020

    Accepted: Apr. 21, 2020

    Posted: Apr. 21, 2020

    Published Online: Jun. 23, 2020

    The Author Email: Jingbi You (jyou@semi.ac.cn)

    DOI: 10.1364/PRJ.392996

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    Yang Zhao, Fei Ma, Feng Gao, Zhigang Yin, Xingwang Zhang, Jingbi You. Research progress in large-area perovskite solar cells[J]. Photonics Research, 2020, 8(7): 070000A1

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  • PEROVSKITE PHOTONICS
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  • Table 1. Photovoltaic Performance of Perovskite Solar Cells Prepared by Different Methods

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    Table 1. Photovoltaic Performance of Perovskite Solar Cells Prepared by Different Methods

    Deposition MethodDevice StructureDevice Area (cm2)PCE (%)Jsc (mA·cm2)Voc (V)FF (%)Reference
    Spin coatingFTO/NiMgLiO/MAPBI3/PCBM/Ti(Nb)Ox/Ag1.0216.220.211.07274.8[17]
    Spin coatingITO/SnO2/(FAPbI3)1x(MAPbBr3)x/Spiro-OMeTAD/Au120.1223.451.1276.85[19]
    Blade coatingITO/PEDOT:PSS/CH3NH3PbIxCl3-x/PC61BM/Bis-C60/Ag10.4416.730.9665.0[28]
    Blade coatingITO/PTAA/MAPbI3/C60/BCP/Cu33.015.019.51.0772.1[21]
    57.215.020.31.0768.9
    Blade coatingITO/PTAA/MAPbI3/C60/BCP/Cu63.716.974.5 (mA)18.976.2[21]
    Slot-die coatingPET/ITO/SnO2/perovskite/Spiro-OMeTAD/Au3014.473.36.5467.0[16]
    Slot-die coatingITO/SnO2/MAPbI3/Spiro-OMeTAD/Au118.021.51.1076.0[30]
    Slot-die coatingITO/ZnO/MAPbI3/doped-P3HT/Ag0.111.619.350.9663.0[31]
    47.34.57
    Slot-die coatingITO/ZnO/MAPbI3/doped-P3HT/Ag0.111.9620.380.9860.0[32]
    Slot-die coatingITO/PEDOT:PSS/MAPbI3/PC61BM/Ca/Ag0.115.7519.791.0277.15[33]
    Slot-die coatingITO/TiO2/CH3NH3PbI3xCl/Spiro-MeOTAD/Au168.7511.10.6921.268.0[34]
    149.511.80.7620.871.0
    Spray coatingITO/PEDOT:PSS/MAPbI3/PCBM/Ca/Al0.02511.116.80.9272.0[36]
    Spray coatingFTO/TiO2/MAPbI3xClx/PTAA/Au4015.584.1 (mA)10.570.16[37]
    Spray coatingITO/TiO2/MAPbI3/Spiro-MeOTAD/Au3.811.719.43.3170.0[35]
    Spray coatingITO/PEDOT:PSS/MAPbI3/C60/BCP/Cu114.221.31.0365.0[38]
    Inkjet printingFTO/TiO2/ZrO2/carbon/perovskite (drop casted perovskite through carbon layer)3110.4619.63.7257.5[41]
    7010.7517.729.6362.9
    Inkjet printingFTO/TiO2/5  nm  C60/MAPbI3/Spiro-MeOTAD/Au413.2420.41.0462.57[42]
    Inkjet printingFTO/c-TiO2/m-TiO2/MAPbI3/Spiro-MeOTAD/Au2.0217.7421.881.0676.5[43]
    Roll-to-rollITO/m-PEDOT:PSS/CH3NH3PbI3/PCBM/Ca/Al6.2511.1617.390.9964.82[34]
    Vacuum-flash-assisted solution processFTO/c-TiO2/m-TiO2/FA0.81MA0.15PbI2.51Br0.45/Spiro-MeOTAD/Au120.3823.191.14376.0[46]
    Pressure-processing methodFTO/c-TiO2/m-TiO2/MAPbI3/Spiro-MeOTAD/Au36.115.771.110.575.7[22]
  • Table 2. Photovoltaic Performance of Perovskite Solar Cells Prepared by Using Different Materials as Additives for Perovskite Layers

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    Table 2. Photovoltaic Performance of Perovskite Solar Cells Prepared by Using Different Materials as Additives for Perovskite Layers

    MaterialsPerovskite ComponentsDevice Area (cm2)PCE (%)Jsc (mA·cm2)Voc (V)FF (%)Reference
    DMSO(FAPbI3)1x(MAPbBr3)x120.1223.451.1276.85[19]
    Nonvolatile coordinating solvents (2-methoxyethanol and acetonitrile)MAPbI363.716.918.974.576.2[29]
    MACl, PbCl2MAPbI3-xClx115.421.01.0669.1[51]
    2512.02.60.79858.2
    MAClMAPbI31.217.3321.381.1172.9[52]
    MAClMAPbI3(Cl)2515.33.666.6563.0[53]
    MAIMAPbI31.215.321.31.0966.1[54]
    PbCl2MAPbI3-xClx413.619.90.9175.0[55]
    KIKx(Cs0.05(FA0.85MA0.15)0.95Pb(I0.85Br0.15)32015.763.576.7965.0[56]
    CsBrCs0.1FA0.9PbI2.9Br0.191.89.341.1613.5559.6[57]
    L-α-phosphatidylcholineMAPbI33315.019.51.0772.1[21]
    57.215.020.31.0768.9
    1,8-diiodooctane (DIO)CH3NH3PbI3xClx10.315.60.9271.0[58]
    1,8-diiodooctane (DIO)CH3NH3PbI3xClx1211.26.482.7163.8[59]
    I3(FAPbI3)x(MAPbBr3)1x119.724.71.1072.3[6]
    PbI2(FAPbI3)1x(MAPbBr3)x120.1223.451.1276.85[19]

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