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Accepted: Apr. 21, 2020

Posted: Apr. 21, 2020

Published Online: Jun. 23, 2020

The Author Email: Jingbi You (jyou@semi.ac.cn)

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Yang Zhao, Fei Ma, Feng Gao, Zhigang Yin, Xingwang Zhang, Jingbi You. Research progress in large-area perovskite solar cells[J]. Photonics Research, 2020, 8(7): 070000A1

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• #### Table 1. Photovoltaic Performance of Perovskite Solar Cells Prepared by Different Methods

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#### Table 1. Photovoltaic Performance of Perovskite Solar Cells Prepared by Different Methods

 Deposition Method Device Structure Device Area ($cm2$) PCE (%) Jsc ($mA·cm−2$) Voc (V) FF (%) Reference Spin coating $FTO/NiMgLiO/MAPBI3/PCBM/Ti(Nb)Ox/Ag$ 1.02 16.2 20.21 1.072 74.8 [17] Spin coating $ITO/SnO2/(FAPbI3)1−x(MAPbBr3)x/Spiro-OMeTAD/Au$ 1 20.12 23.45 1.12 76.85 [19] Blade coating $ITO/PEDOT:PSS/CH3NH3PbIxCl3-x/PC61BM/Bis-C60/Ag$ — 10.44 16.73 0.96 65.0 [28] Blade coating $ITO/PTAA/MAPbI3/C60/BCP/Cu$ 33.0 15.0 19.5 1.07 72.1 [21] 57.2 15.0 20.3 1.07 68.9 Blade coating $ITO/PTAA/MAPbI3/C60/BCP/Cu$ 63.7 16.9 74.5 (mA) 18.9 76.2 [21] Slot-die coating $PET/ITO/SnO2/perovskite/Spiro-OMeTAD/Au$ 30 14.47 3.3 6.54 67.0 [16] Slot-die coating $ITO/SnO2/MAPbI3/Spiro-OMeTAD/Au$ 1 18.0 21.5 1.10 76.0 [30] Slot-die coating $ITO/ZnO/MAPbI3/doped-P3HT/Ag$ 0.1 11.6 19.35 0.96 63.0 [31] 47.3 4.57 — — — Slot-die coating $ITO/ZnO/MAPbI3/doped-P3HT/Ag$ 0.1 11.96 20.38 0.98 60.0 [32] Slot-die coating $ITO/PEDOT:PSS/MAPbI3/PC61BM/Ca/Ag$ 0.1 15.75 19.79 1.02 77.15 [33] Slot-die coating $ITO/TiO2/CH3NH3PbI3−xCl/Spiro-MeOTAD/Au$ 168.75 11.1 0.69 21.2 68.0 [34] 149.5 11.8 0.76 20.8 71.0 Spray coating $ITO/PEDOT:PSS/MAPbI3/PCBM/Ca/Al$ 0.025 11.1 16.8 0.92 72.0 [36] Spray coating $FTO/TiO2/MAPbI3−xClx/PTAA/Au$ 40 15.5 84.1 (mA) 10.5 70.16 [37] Spray coating $ITO/TiO2/MAPbI3/Spiro-MeOTAD/Au$ 3.8 11.7 19.4 3.31 70.0 [35] Spray coating $ITO/PEDOT:PSS/MAPbI3/C60/BCP/Cu$ 1 14.2 21.3 1.03 65.0 [38] Inkjet printing $FTO/TiO2/ZrO2/carbon/perovskite$ (drop casted perovskite through carbon layer) 31 10.46 19.6 3.72 57.5 [41] 70 10.75 17.72 9.63 62.9 Inkjet printing $FTO/TiO2/5 nm C60/MAPbI3/Spiro-MeOTAD/Au$ 4 13.24 20.4 1.04 62.57 [42] Inkjet printing $FTO/c-TiO2/m-TiO2/MAPbI3/Spiro-MeOTAD/Au$ 2.02 17.74 21.88 1.06 76.5 [43] Roll-to-roll $ITO/m-PEDOT:PSS/CH3NH3PbI3/PCBM/Ca/Al$ 6.25 11.16 17.39 0.99 64.82 [34] Vacuum-flash-assisted solution process $FTO/c-TiO2/m-TiO2/FA0.81MA0.15PbI2.51Br0.45/Spiro-MeOTAD/Au$ 1 20.38 23.19 1.143 76.0 [46] Pressure-processing method $FTO/c-TiO2/m-TiO2/MAPbI3/Spiro-MeOTAD/Au$ 36.1 15.7 71.1 10.5 75.7 [22]
• #### Table 2. Photovoltaic Performance of Perovskite Solar Cells Prepared by Using Different Materials as Additives for Perovskite Layers

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#### Table 2. Photovoltaic Performance of Perovskite Solar Cells Prepared by Using Different Materials as Additives for Perovskite Layers

 Materials Perovskite Components Device Area ($cm2$) PCE (%) Jsc ($mA·cm−2$) Voc (V) FF (%) Reference DMSO $(FAPbI3)1−x(MAPbBr3)x$ 1 20.12 23.45 1.12 76.85 [19] Nonvolatile coordinating solvents (2-methoxyethanol and acetonitrile) $MAPbI3$ 63.7 16.9 18.9 74.5 76.2 [29] MACl, $PbCl2$ $MAPbI3-xClx$ 1 15.4 21.0 1.06 69.1 [51] 25 12.0 2.6 0.798 58.2 MACl $MAPbI3$ 1.2 17.33 21.38 1.11 72.9 [52] MACl $MAPbI3(Cl)$ 25 15.3 3.66 6.65 63.0 [53] MAI $MAPbI3$ 1.2 15.3 21.3 1.09 66.1 [54] $PbCl2$ $MAPbI3-xClx$ 4 13.6 19.9 0.91 75.0 [55] KI $Kx(Cs0.05(FA0.85MA0.15)0.95Pb(I0.85Br0.15)3$ 20 15.76 3.57 6.79 65.0 [56] CsBr $Cs0.1FA0.9PbI2.9Br0.1$ 91.8 9.34 1.16 13.55 59.6 [57] L-$α$-phosphatidylcholine $MAPbI3$ 33 15.0 19.5 1.07 72.1 [21] 57.2 15.0 20.3 1.07 68.9 1,8-diiodooctane (DIO) $CH3NH3PbI3−xClx$ — 10.3 15.6 0.92 71.0 [58] 1,8-diiodooctane (DIO) $CH3NH3PbI3−xClx$ 12 11.2 6.48 2.71 63.8 [59] $I3−$ $(FAPbI3)x(MAPbBr3)1−x$ 1 19.7 24.7 1.10 72.3 [6] $PbI2$ $(FAPbI3)1−x(MAPbBr3)x$ 1 20.12 23.45 1.12 76.85 [19]